Hybrid Catalysts for CO2 Conversion into Cyclic Carbonates

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3 Citazioni (Scopus)

Abstract

The conversion of carbon dioxide into valuable chemicals such as cyclic carbonates is an appealing topic for the scientific community due to the possibility of valorizing waste into an inexpensive, available, nontoxic, and renewable carbon feedstock. In this regard, last-generation heterogeneous catalysts are of great interest owing to their high catalytic activity, robustness, and easy recovery and recycling. In the present review, recent advances on CO2 cycloaddition to epoxide mediated by hybrid catalysts through organometallic or organo-catalytic species supported onto silica-, nanocarbon-, and metal-organic framework (MOF)-based heterogeneous materials, are highlighted and discussed.
Lingua originaleEnglish
pagine (da-a)325-
Numero di pagine30
RivistaCatalysts
Volume9
Stato di pubblicazionePublished - 2019

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title = "Hybrid Catalysts for CO2 Conversion into Cyclic Carbonates",
abstract = "The conversion of carbon dioxide into valuable chemicals such as cyclic carbonates is an appealing topic for the scientific community due to the possibility of valorizing waste into an inexpensive, available, nontoxic, and renewable carbon feedstock. In this regard, last-generation heterogeneous catalysts are of great interest owing to their high catalytic activity, robustness, and easy recovery and recycling. In the present review, recent advances on CO2 cycloaddition to epoxide mediated by hybrid catalysts through organometallic or organo-catalytic species supported onto silica-, nanocarbon-, and metal-organic framework (MOF)-based heterogeneous materials, are highlighted and discussed.",
keywords = "carbon dioxide; cyclic carbonate; heterogeneous catalysis; ionic liquids; carbon nanotubes; fullerene; graphene; MOF",
author = "Francesco Giacalone and Carmela Aprile and Carla Calabrese",
year = "2019",
language = "English",
volume = "9",
pages = "325--",
journal = "Catalysts",
issn = "2073-4344",
publisher = "Multidisciplinary Digital Publishing Institute (MDPI)",

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T1 - Hybrid Catalysts for CO2 Conversion into Cyclic Carbonates

AU - Giacalone, Francesco

AU - Aprile, Carmela

AU - Calabrese, Carla

PY - 2019

Y1 - 2019

N2 - The conversion of carbon dioxide into valuable chemicals such as cyclic carbonates is an appealing topic for the scientific community due to the possibility of valorizing waste into an inexpensive, available, nontoxic, and renewable carbon feedstock. In this regard, last-generation heterogeneous catalysts are of great interest owing to their high catalytic activity, robustness, and easy recovery and recycling. In the present review, recent advances on CO2 cycloaddition to epoxide mediated by hybrid catalysts through organometallic or organo-catalytic species supported onto silica-, nanocarbon-, and metal-organic framework (MOF)-based heterogeneous materials, are highlighted and discussed.

AB - The conversion of carbon dioxide into valuable chemicals such as cyclic carbonates is an appealing topic for the scientific community due to the possibility of valorizing waste into an inexpensive, available, nontoxic, and renewable carbon feedstock. In this regard, last-generation heterogeneous catalysts are of great interest owing to their high catalytic activity, robustness, and easy recovery and recycling. In the present review, recent advances on CO2 cycloaddition to epoxide mediated by hybrid catalysts through organometallic or organo-catalytic species supported onto silica-, nanocarbon-, and metal-organic framework (MOF)-based heterogeneous materials, are highlighted and discussed.

KW - carbon dioxide; cyclic carbonate; heterogeneous catalysis; ionic liquids; carbon nanotubes; fullerene; graphene; MOF

UR - http://hdl.handle.net/10447/357450

M3 - Article

VL - 9

SP - 325-

JO - Catalysts

JF - Catalysts

SN - 2073-4344

ER -