CO2 conversion in a photocatalytic continuous membrane reactor

Marianna Bellardita, Leonardo Palmisano, Brunetti, Drioli, Sellaro, Fontananova, Barbieri

Research output: Contribution to journalArticlepeer-review

18 Citations (Scopus)

Abstract

The reduction of CO2 with water by using photocatalysts is one of the most promising new methods for achieving CO2 conversion to valuable hydrocarbons such as methanol (MeOH). In this work, prepared TiO2-Nafion™-based membranes were used in a photocatalytic membrane reactor, operated in continuous mode, for converting CO2 to methanol. By using the membrane with the best TiO2 distribution, a MeOH flow rate/TiO2 weight of 45 μmol (gcatalyst h)-1 was measured when operating at 2 bar of feed pressure. This value is higher than those reported in most of the literature data to date. Moreover, methanol production is considered as a relevant advance over the existing literature results which mostly propose CH4 as the reaction product.
Original languageEnglish
Pages (from-to)67418-67427
Number of pages10
JournalRSC Advances
Volume6
Publication statusPublished - 2016

All Science Journal Classification (ASJC) codes

  • General Chemistry
  • General Chemical Engineering

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